How to fix "Only one expression can be specified in the select list when the subquery is not introduced with EXISTS" error?

Try this one -

"SELECT 
       ID, Salt, password, BannedEndDate
     , (
          SELECT COUNT(1)
          FROM dbo.LoginFails l
          WHERE l.UserName = u.UserName
               AND IP = '" + Request.ServerVariables["REMOTE_ADDR"] + "'
      ) AS cnt
FROM dbo.Users u
WHERE u.UserName = '" + LoginModel.Username + "'"

Try this:

 Select 
    Id, 
    Salt, 
    Password, 
    BannedEndDate, 
    (Select Count(*) 
        From LoginFails 
        Where username = '" + LoginModel.Username + "' And IP = '" + Request.ServerVariables["REMOTE_ADDR"] + "')
 From Users 
 Where username = '" + LoginModel.Username + "'

And I recommend you strongly to use parameters in your query to avoid security risks with sql injection attacks!

Hope that helps!